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<article language="en">
	<journal>
		<journal_title>Geoscientific Model Development Discussions</journal_title>
		<journal_url>www.geosci-model-dev-discuss.net</journal_url>
		<issn>1991-9611</issn>
		<eissn>1991-962X</eissn>
		<volume_number>2</volume_number>
		<issue_number>2</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/gmdd-2-681-2009</doi>
	<article_url>http://www.geosci-model-dev-discuss.net/2/681/2009/</article_url>
	<abstract_html>http://www.geosci-model-dev-discuss.net/2/681/2009/gmdd-2-681-2009.html</abstract_html>
	<fulltext_pdf>http://www.geosci-model-dev-discuss.net/2/681/2009/gmdd-2-681-2009.pdf</fulltext_pdf>
	<start_page>681</start_page>
	<end_page>707</end_page>
	<publication_date>2009-07-01</publication_date>
	<article_title content_type="html">Implementation of a new aerosol HAM model within the Weather Research and Forecasting (WRF) modeling system</article_title>
	<authors>
		<author numeration="1" affiliations="1,2">
			<name>R. Mashayekhi</name>
			<email>rmash@ut.ac.ir</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>P. Irannejad</name>
		</author>
		<author numeration="3" affiliations="2">
			<name>J. Feichter</name>
		</author>
		<author numeration="4" affiliations="1">
			<name>A. A. Bidokhti</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Institute of Geophysics, University of Tehran, Tehran, Iran</affiliation>
		<affiliation numeration="2" content_type="html">Max Planck Institute for Meteorology, Hamburg, Germany</affiliation>
	</affiliations>
	<abstract content_type="html">A new coupled system of aerosol HAM model and the Weather, Research and
Forecasting (WRF) model is presented in this paper. Unlike the current
aerosol schemes used in WRF model, the HAM is using a &quot;pseudomodal&quot;
approach for the representation of the particle size distribution. The
aerosol components considered are sulfate, black carbon, particulate organic
matter, sea salt and mineral dust. The preliminary model results are
presented for two different 6-day simulation periods from 22 to 28 February
2006 as a winter period and 6 to 12 May 2006 as a mild period. The mean
shortwave radiation and thermal forcing were calculated from the model
simulations with and without aerosols feedback for two simulation periods. A
negative radiative forcing and cooling of the atmosphere were found mainly
over the regions of high emission of mineral dust. The absorption of
shortwave radiation by black carbon caused warming effects in some regions
with positive radiative forcing. The simulated daily mean sulfate mass
concentration showed a rather good agreement with the measurements in the
European EMEP network. The diurnal variation of the simulated hourly
PM&lt;sub&gt;10&lt;/sub&gt; mass concentration at Tehran was also qualitatively close to the
observations in both simulation periods. The model captured diurnal cycle and
the magnitude of the observed PM&lt;sub&gt;10&lt;/sub&gt; concentration during most of the
simulation periods. The differences between the observed and simulated
PM&lt;sub&gt;10&lt;/sub&gt; concentration resulted mostly from limitation of the model in
simulating the clouds and precipitation, transport errors and uncertainties
in the particulate emission rates. The inclusion of aerosols feedback in
shortwave radiation scheme improved the simulated daily mean shortwave
radiation fluxes in Tehran for both simulation periods.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Ackermann, I. J., Hass, H., Memmesheimer, M., Ebel, E., Binkowski, F. S., and Shankar, U.: Modal aerosol dynamics model for Europe: Development and first applications, Atmos. Environ., 32, 2981–2999, 1998. </reference>
		<reference numeration="2" content_type="text"> Albrecht, B. A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227–1230, 1989. </reference>
		<reference numeration="3" content_type="text"> Barnard, J. C., Chapman, E. G., Fast, J. D., Schemlzer, J. R., Slusser, J. R., and Shetter, R. E.: An evaluation of the FAST–J photolysis algorithm for predicting Nitrogen Dioxide photolysis rates under clear and cloudy sky conditions, Atmos, Environ., 38, 3393–3403, 2004a. </reference>
		<reference numeration="4" content_type="text"> Chang, J. S., Binkowski, F. S., Seaman, N. L., McHenry, J. N., Samson, P. J., Stockwell, W. R., Walcek, C. J., Madornich, S., Middleton, P. B., Pleim, J. E., and Lansford, H. H.: The regional acid deposition model and engineering model, state-of-science/Technology, Report 4, National Acid Precipitation Assessment Program, Washington DC, 1989. </reference>
		<reference numeration="5" content_type="text"> Charlson, R. J., Lovelock, J. E., Andreae, M. O., and Warren, S. G.: Oceanic phytoplankton, atmospheric sulfur, cloud albedo and climate, Nature, 326, 655–661, 1987. </reference>
		<reference numeration="6" content_type="text"> Charlson, R. J., Schwartz, S. E., Hales, J. M., Cess, R. D., Coakley Jr., J. A., Hansen, J. E., and Hofmann, D. J.: Climate forcing by anthropogenic aerosols, Science, 255, 423–430, 1992. </reference>
		<reference numeration="7" content_type="text"> Chou, M. D., Suarez, M. J., Ho, C. H., Yan, M. H. H., and Lee, K. T.: Parameterizations for cloud overlapping and shortwave single-scattering properties for use in general circulation and cloud ensemble models, J. Climate, 11, 202–214, 1998. </reference>
		<reference numeration="8" content_type="text"> Dentener, F., Kinne, S., Bond, T., Boucher, O., Cofala, J., Generoso, S., Ginoux, P., Gong, S., Hoelzmann, J. J., Ito, A., Marelli, L., Penner, J. E., Putaud, J. P., Textor, C., Schulz, M., Van der Werf, J. R., and Wilson, J.: Emissions of primary aerosol and precursor gases in the years 2000 and 1750 orescribed data-sets for AeroCom, J. Atmos. Chem. Phys., 6, 4321–4344, 2006. </reference>
		<reference numeration="9" content_type="text"> Fast, J. D., Gustafson, W. I., Easter Jr., R. C., Zaveri, R. A., Barnard, J. C., Chapman, E. G., Grell, G. A., and Peckham, S. E.: Evolution of ozone, particulates, and aerosol direct radiative forcing in the vicinity of Houston using a fully coupled meteorology-chemistry-aerosol model, J. Geophys. Res., 111, D21305, doi:10.1029/2005JD006721, 2006. </reference>
		<reference numeration="10" content_type="text"> Fuchs, N. A.: Evaporation and Droplet Growth in Gaseous Media, Pergamon, Tarrytown, New York, 72~pp., 1959. </reference>
		<reference numeration="11" content_type="text"> Fuchs, N. A.: The Mechanics of Aerosols, Pergamon press, Oxford, 1964. </reference>
		<reference numeration="12" content_type="text"> Gong, S. L., Barriel, A., and Lazare, M.: Canadanian Aerosol Module: A size-segregated simulation of atmospheric aerosol processes for climate and air quality models: 1. Module development, J. Geophys. Res., 108(D1), 4007, doi:10.1029/2001JD002002, 2003. </reference>
		<reference numeration="13" content_type="text"> Grell, G. A. and Devenyi, D.: A generalized approach to parameterizing convection combining ensemble and data assimilation techniques, Geophys. Res. Lett., 29(14), 38.1–38.4 2002. </reference>
		<reference numeration="14" content_type="text"> Grell, G. A., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully coupled &quot;online&quot; chemistry within the WRF model, Atmos. Environ., 39, 6957–6975, 2005. </reference>
		<reference numeration="15" content_type="text"> Hong, S. Y., Noh, Y., and Dudhia, J.: A new vertical diffusion package with an explicit treatment of entrainment processes, Mon. Weather Rev., 134, 2318–2341, 2006. </reference>
		<reference numeration="16" content_type="text"> IPCC, Climate Change 2007 – The Physical Science Basis, contribution of the Working Group I to the forth assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, K. B., Tignor, M., and Miller, H. L., Cambridge Univ. Press, Cambridge, United Kingdom and New York, NY, USA, 2007. </reference>
		<reference numeration="17" content_type="text"> Jacobson, M. Z.: Global direct radiative forcing due to muticomponent anthropogenic and natural aerosols, J. Geophys. Res., 106, 1551–1568, 2001. </reference>
		<reference numeration="18" content_type="text"> Kulmala, M., Laaksonen, A., and Pirjola, L.: Parameterizations for sulfuric acid/water nucleation rates, J. Geophys. Res., 103, 8301–8307, 1998. </reference>
		<reference numeration="19" content_type="text"> Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S. A.: Radiative transfer for inhomogeneous atmosphere: RRTM, a validated correlated-K model for longwave, J. Geophys. Res., 102, 16 663–16 682, 1997. </reference>
		<reference numeration="20" content_type="text"> Monin, A. S. and Obukhov, A. M.: Basic laws of turbulent mixing in the ground layer of the atmosphere, Trans. Geophys. Inst. Akad. Nauk USSR, 151, 163–187, 1954. </reference>
		<reference numeration="21" content_type="text"> Pleim, J. E., Venkatram, A., and Yamartino, R.: ADOM/TADAP Model Development Program, Vol 4, The Dry Deposition Module, Ontario Ministry of the Environment, Canada, 1984. </reference>
		<reference numeration="22" content_type="text"> Ramanathan, V. and Vogelmann, A. M.: Greenhouse effect, atmospheric solar absorption, and the Earth&apos;s radiation budget: From the Arrhenius-Langely era to the 1990&apos;s, Ambio, 26(1), 38–46, 1997. </reference>
		<reference numeration="23" content_type="text"> Ramanathan, V., Crutzen, P. J., Kiehl, J. T., and Rosenfeld, D.: Aerosols, climate, and the hydrological cycle, Science, 294, 2119–2124, 2001a. </reference>
		<reference numeration="24" content_type="text"> Ramanathan, V.: Indian Ocean Exprement: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze, J. Geophys, Res., 106, 28 371–28 398, 2001b. </reference>
		<reference numeration="25" content_type="text"> Rodriguez, M. A. and Dabdub, D.: IMAGES-SCAPE2: A modeling study of size- and chemistry resolved aerosol thermodynamics in a global chemical transport model, J. Geophys. Res., 109, D02203, doi:10.1029/2003JD003639, 2004. </reference>
		<reference numeration="26" content_type="text"> Schell B., Ackermann, I. J., Hass, H., Binkowski, F. S., and Ebel, A.: Modeling the formation of secondary organic aerosol within a comprehensive air quality model system, J. Geophys. Res., 106, 28 275–28 293, 2001. </reference>
		<reference numeration="27" content_type="text"> Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D. M., Wang, W., and Powers, J. G.: A description of the Advanced Research WRF version 2, NCAR Tech Note, NCAR/TN468+STR, 88~pp., 2005. </reference>
		<reference numeration="28" content_type="text"> Slinn, S. A. and Slinn, W. G. N.: Predictions for particle deposition on natural waters, Atmos. Environ., 14, 1013–1016, 1980. </reference>
		<reference numeration="29" content_type="text"> Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, 2005. </reference>
		<reference numeration="30" content_type="text"> Twomey, S.: Aerosols, clouds and radiation, Atmos. Environ A-Gen., 25, 2435–2442, 1991. </reference>
		<reference numeration="31" content_type="text"> Vehkamaki, H., Kulmala, M., Napari, I., Lehtinen, K. E. J., Timmreck, C., Noppel, M., and Laaksonen, A.: An improved parameterization for sulfuric acid-water nucleation rates for tropospheric and stratospheric conditions, J. Geophys. Res., 107(D22), 4622, doi:10.1029/2002JD002184, 2002. </reference>
		<reference numeration="32" content_type="text"> Vignati, E., Wilson, J., and Stier, P.: M7: a size resolved aerosol mixture module for the use in global aerosol models, J. Geophys. Res., 109, D22202, doi:10.1029/2003JD004485, 2004. </reference>
		<reference numeration="33" content_type="text"> Whitby, E. R. and McMurry, P. H.: Modal aerosol dynamics modeling, Aerosol Sci. Technol., 27, 673–688, 1997. </reference>
		<reference numeration="34" content_type="text"> Wild, O., Zhu, X., and Prather, M. J.: Fast-J: Accurate simulation of in- and bellow-cloud photolysis in tropospheric chemical models, J. Atmos. Chem., 37, 245–282, 2000. </reference>
		<reference numeration="35" content_type="text"> Williams, M. M. R., and Loyalka, S. K.: Aerosol Science: Theory and Practice, Pergamon, New York, 1991. </reference>
		<reference numeration="36" content_type="text"> Wilson, J., Cuvelier, C., and Raes, F.: A modeling study of global mixed aerosol fields, J. Geophys. Res., 106, 34 081–34 108, 2001. </reference>
		<reference numeration="37" content_type="text"> Wesely, M. L.: Parameterization of surface resistance to gaseous dry deposition in regional numerical models, Atmos. Environ., 16, 1293–1304, 1989. </reference>
		<reference numeration="38" content_type="text"> Zaveri, R. A., Easter, R. C., and Wexler, A. S.: A new method for multicomponent activity coefficients of electrolytes in aqueous atmospheric aerosols, J. Geophys. Res., 110, D02201, doi:10.1029/2004JD004681, 2005a. </reference>
		<reference numeration="39" content_type="text"> Zaveri, R. A., Easter, R. C., and Peters, L. K.: A computationally efficient Multicomponent Equilibrium Solver for Aerosols (MESA), J. Geophys. Res., 110, D24203, doi:10.1029/2004JD005618, 2005b. </reference>
	</references>
</article>

